This is the Police Headquarters Building located at 240 Centre Street. Designed by the firm of Hoppin & Koen in an exuberant Edwardian Baroque style, it opened in 1909. The NYPD moved out in 1973 and it was converted to luxury condominiums in 1987. There are 55 apartments on six floors. 2-bedroom rents ranging from $7,000 – $11,500 & 2-bedroom sale ranging from $1.05M (1,750 sq. ft.) – $1.5M. Read more about it here.